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人工甜味剂在污水处理厂和自来水厂的归趋
  • ISSN号:1001-6929
  • 期刊名称:《环境科学研究》
  • 时间:0
  • 分类:X131.2[环境科学与工程—环境科学]
  • 作者机构:[1]南开大学环境科学与工程学院,环境污染过程与基准教育部重点实验室,天津300071
  • 相关基金:国家自然科学基金项目(41073087)
中文摘要:

研究了7种常用的人工甜味剂〔安赛蜜、三氯蔗糖、糖精、甜蜜素、纽甜、阿斯巴甜和NHDC(新橙皮苷二氢查耳酮)〕在污水处理厂及自来水厂的分布.7种人工甜味剂在污水处理厂进水中均被检出,质量浓度为6.4~31 671.0 ng/L.安赛蜜、三氯蔗糖、糖精、甜蜜素在污水处理厂的出水中被检出,质量浓度为32.4~11 204.0 ng/L.这些甜味剂将随污水处理厂的出水排放而进入水环境.安赛蜜、三氯蔗糖、糖精、甜蜜素、纽甜在自来水厂进水中被检出,质量浓度为低于定量限~579.4 ng/L,其中前4种在自来水中被检出,质量浓度为23.3~504.2 ng/L.沉淀、絮凝、氯化消毒作用对人工甜味剂没有明显的去除作用.生物降解能有效去除糖精、甜蜜素、阿斯巴甜、纽甜和NHDC,但对安赛蜜和三氯蔗糖去除率不高,去除率均小于20%.

英文摘要:

The occurrence and removal of seven commonly used artificial sweeteners, including acesulfame, sucralose, saccharin, cyclamate, neotame, aspartame and neohesperidin dihydrochalcone (NHDC) in waste water treatment processes (WWTP) and drinking water treatment processes (DWTP) were assessed. All of the seven investigated artificial sweeteners were detected in the influent of WWTP, with concentrations ranging from 6.4-31,671.0 ng/L. The first four artificial sweeteners ( acesulfame, sucralose, saccharin and cyclamate) were detected in the effluent, with concentrations ranging from 32.4-11,204.0 ng/L. They might be a contaminant source for surface water. Acesulfame, sucralose, saccharin, cyclamate and neotame were found in the source water of DWTP, with concentrations between 〈 LOQ and 579.4 ng/L. The first four artificial sweeteners were detected in drinking water, with concentrations ranging from 23.3-504. 2 ng/L. The sedimentation, floeculation and chlorination in DWTP could not significantly remove the investigated artificial sweeteners. Compared with the other five artificial sweeteners ( saccharin, cyclamate, aspartame, neotame and NHDC) , sueralose and acesulfame were found to be very persistent against microbial degradation; their elimination rates in WWTP were less than 20%.

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期刊信息
  • 《环境科学研究》
  • 中国科技核心期刊
  • 主管单位:中华人民共和国环境保护部
  • 主办单位:中国环境科学研究院
  • 主编:刘鸿亮
  • 地址:北京安外大羊坊8号中国环科院内
  • 邮编:100012
  • 邮箱:hjkxyj@163.com
  • 电话:010-84915128
  • 国际标准刊号:ISSN:1001-6929
  • 国内统一刊号:ISSN:11-1827/X
  • 邮发代号:82-384
  • 获奖情况:
  • 国内外数据库收录:
  • 俄罗斯文摘杂志,美国化学文摘(网络版),英国农业与生物科学研究中心文摘,波兰哥白尼索引,荷兰文摘与引文数据库,美国工程索引,美国剑桥科学文摘,英国动物学记录,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国国家哲学社会科学学术期刊数据库,中国北大核心期刊(2000版)
  • 被引量:33433