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热电材料PbTel-xSex的高压制备及电学性能研究
  • ISSN号：1000-5773
  • 期刊名称：《高压物理学报》
  • 时间：0
  • 分类：O521.2[理学—高压高温物理;理学—物理]
  • 作者机构：[1]河南理工大学材料科学与工程学院,河南焦作454003, [2]河南理工大学物理化学学院,河南焦作454003, [3]上海出入境检验检疫局,上海200135, [4]吉林大学超硬材料国家重点实验室,吉林长春130012
  • 相关基金：国家自然科学基金重点项目（50731006）;国家自然科学基金青年科学基金项目（51001042,50801030）;河南理工大学博士基金（B2010-55）;吉林大学超硬材料国家重点实验室开放课题（201005）
作者： 宿太超[1], 朱红玉[2], 李洪涛[3], 李尚升[1], 李小雷[1], 马红安[4], 贾晓鹏[1,4]
关键词： 高压, 热电材料, PbTe1-xSex, high pressure thermoelectric material PbTe1-xSex
中文摘要：

利用高温高压技术，制备了热电材料PbTe和PbSe的固溶体合金PbTe1-xSex，在室温下对其结构及电学性质进行了研究。X射线衍射（XRD）测试结果表明：PbTe1-xSex具有NaCl结构；晶格常数随着Se含量（x）的增加而减小；PbTe1-xSex的电阻率和Seebeck系数的绝对值随x的增大而减小；功率因子随x的增大先增大而后减小，当x=0.1时功率因子最高，达到21.7 μW/（cm·K2），比相同条件下制备的PbTe高20%。

英文摘要：

The n-type thermoelectric materials of PbTe alloyed with PbSe （PbTe1-xSex） were prepared by high-pressure and high-temperature method. The structure and electrical properties of PbTe1-xSex were studied at room temperature. X-ray diffraction results indicated that the PbTe1-xSex sample exhibited the NaCl crystal structure. As the increasing of Se content x, the lattice parameter, Seebeck coefficient and resistivity for PbTe1-xSex all decrease, and the power factor increases first and then decreases. The maximum power factor of 21.7 μW/（cm·K2） was obtained at the x=0.1, which is about 20% higher than that of PbTe.

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期刊信息
  • 《高压物理学报》
  • 北大核心期刊（2011版）
  • 主管单位:四川省科学技术协会
  • 主办单位:中国物理学会 高压物理专业委员会 四川省物理学会
  • 主编：邹广田
  • 地址：四川省绵阳市919信箱110分箱
  • 邮编：621999
  • 邮箱：gaoya@caep.cn
  • 电话：0816-2490042
  • 国际标准刊号：ISSN：1000-5773
  • 国内统一刊号：ISSN：51-1147/O4
  • 邮发代号:62-132
  • 获奖情况:
  • 中国物理类核心期刊,EI、CI收录期刊,中国期刊方阵“双效”期刊
  • 国内外数据库收录:
  • 美国化学文摘（网络版）,荷兰文摘与引文数据库,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊（2004版）,中国北大核心期刊（2008版）,中国北大核心期刊（2011版）,中国北大核心期刊（2014版）,中国北大核心期刊（2000版）
  • 被引量:3617