基于作者构造的He-HBr体系的各向异性势,采用密耦方法计算了碰撞能量分别为60和100 meV时3He、4He、6He和7He被HBr分子散射的角分布,详细讨论了氦同位素对散射角分布的影响.结果表明:在相同碰撞能量时,随着同位素氦原子质量的增加,总微分截面在0°时的角分布逐渐增大,同一级衍射振荡极小值位置逐渐向小散射角方向移动;弹性与总非弹性截面交界角逐渐减小,总非弹性截面逐渐增加.碰撞能量越低,入射同位素He原子的质量越大,彩虹现象越明显.
Angular distribution for scatterings of ^3He,^4He,^6He and ^7He with hydrogen bromide molecules are calculated by using close-coupling approach from the anisotropic intermolecular potential of the He-HBr system established by the author. The calculations are performed separately at the collision energies of 60 and 100 meV. The influences of He isotope atoms on angular distribution is discussed in detail. The results show that the angular distribution of the total differential cross section (DCS) at zero degree increases and the position of oscillation minimum of the same order gradually shift towards small scattering angle along with the increase of the incident isotope He atom mass at identical collision energy. And crossing angle between the elastic and total inelastic DCS gradually decreases and the total inelastic DCS gradually increases. The rainbow phenomenon become more evident for the lower the collision energy and the larger mass of the incident He isotope atom.