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Key features of new particle formation events at background sites in China and their influence on cloud condensation nuclei
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  • 分类:P402[天文地球—大气物理学与大气环境;天文地球—大气科学及气象学]
  • 作者机构:[1]中国气象科学研究院灾害天气国家重点实验室/中国气象局大气化学重点开放实验室,北京100081, [2]中国科学院寒区旱区环境与工程研究所冰冻圈科学国家重点实验室,甘肃兰州730000, [3]山东大学环境研究院,山东济南250100
  • 相关基金:中国极地科学战略研究基金项目(20140310); 国家自然科学基金(41175113;41405132)资助
中文摘要:

2013年9月在北极黄河站开展了气溶胶数谱(10~400 nm)的短期观测实验.数浓度小时平均值主要出现在300~400 cm^-3,平均值为350 cm^-3,高于新奥尔松Zeppelin全球大气本底站及环北极海洋大气7-9月航测报道的浓度.大气气溶胶的三个模态(核模态、爱根核模态和积聚模态)数浓度平均分别为35、122和193 cm^-3.观测期间没有发生新粒子生成事件,平均数谱分布呈现双模态的分布特征,模态峰值分别出现在30 nm和115 nm,由积聚模态主导.平均数谱分布的几何中值粒径出现在约100~110 nm.从单颗粒分析结果来看,观测期间黄河站地区大气气溶胶主要以海盐气溶胶为主,但是在来自挪威海域和北欧大陆的气团影响下,也观测到煤烟颗粒、富硫颗粒物和含碳颗粒物等人为气溶胶.

英文摘要:

Measurement of particle number size distribution(PNSD)in the size range of 10 ~ 400 nm was carried out at Yellow River Station in Arctic in September 2013. During the measurement,it was found that the value of hourly mean number concentration of 300 ~ 400 cm^-3 presented most frequently,with a mean value of 350cm^-3. The number concentration was much higher than the values reported by the study at Zeppelin Station in Ny-?lesund and the cruises in the central Arctic between July and September. The number concentration of the three modes(nucleation mode,Aitken mode and accumulation mode)was 35,122 and 193 cm^-3,respectively. There was no new particle formation event observed during the measurement. The PNSD was characterized by bimodal distribution,with one mode peaking at 30 nm and the other at 115 nm,respectively. The PNSD was dominated by the accumulation mode,with the geometric mean diameter of 100 ~ 110 nm. Based on the analysis of the individual particle samples,it was found that the chemical component during the measurement was mainly contributed by the sea salt particles. However,when air mass from Norwegian Sea and Northern Europe became dominant,the soot particles,sulfur- rich and carbonaceous particles were also observed,revealing the influence by the anthropogenic emissions.

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