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Self-assembly of Hydrazide-based Heterodimers Driven by Hydrogen Bonding and Donor-Acceptor Interaction
  • ISSN号：1001-604X
  • 期刊名称：《中国化学：英文版》
  • 时间：0
  • 分类：O623.752[理学—有机化学;理学—化学]
  • 作者机构：[1]Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai 200032, China
  • 相关基金：Project supportecl by the National Natural Science Foundation of China （Nos. 20321202. 20332040. 20425208）. Dedicated to Professor Xikui Jiang on the occasion of his 80th birthday.
作者： 冯代军[1], 王鹏[1], 李小强[1], 黎占亭[1]
关键词： 酰肼, 异质二聚物, 自组装, 氢键结合, 供体-受体相互作用, hydrazide, heterodimer, self-assembly, hydrogen bonding, donor-acceptor interaction
中文摘要：

氢的一个新系列契约驱动的 heterodimers 在从基于一种肺结核特效药的单体的氯仿自我装配。在充满电子的二度(p苯撑)之间的另外的分子间的施主领受人相互作用联合起来的 -34-crown-10 和联合起来的电子缺乏的萘 diimide 被利用了增加 dimmers 的稳定性，并且二分离非共有原子价的显著 cooperativity 强迫稳定更暗淡被量的 1H ( 2D )揭示了 NMR 和紫外力的实验。

英文摘要：

A new series of hydrogen bonding-driven heterodimers have been self-assembled in chloroform from hydrazide-based monomers. Additional intermolecular donor-acceptor interaction between the electron-rich bis（p-phenylene）-34-crown-10 unit and the electron-deficient naphthalene diimide unit has been utilized to increase the stability of the dimmers, and pronounced cooperativity of the two discrete non-covalent forces to stabilize the dimer has been revealed by the quantitative ^1H （2D） NMR and UV-Vis experiments.

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期刊信息
  • 《中国化学：英文版》
  • 主管单位:
  • 主办单位:中国化学会
  • 主编：
  • 地址：上海市枫林路354号中科院上海有机化学研究所
  • 邮编：200032
  • 邮箱：
  • 电话：021-54925243
  • 国际标准刊号：ISSN：1001-604X
  • 国内统一刊号：ISSN：31-1547/O6
  • 邮发代号:4-646
  • 获奖情况:
  • 中国期刊方阵“双高”期刊
  • 国内外数据库收录:
  • 美国化学文摘（网络版）,荷兰文摘与引文数据库,美国科学引文索引（扩展库）,日本日本科学技术振兴机构数据库,英国英国皇家化学学会文摘
  • 被引量:175