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西安郊区泾河秋、冬季大气黑碳变化及粒径特征
  • ISSN号:1001-6929
  • 期刊名称:《环境科学研究》
  • 时间:0
  • 分类:X51[环境科学与工程—环境工程]
  • 作者机构:[1]陕西省气象科研所,陕西西安710015
  • 相关基金:国家公益性行业(气象)专项(GYHY201306005); 中国气象局气候变化专项(CCSF201327); 国家重点基础研究发展计划(973)项目(2013CB955800)
中文摘要:

利用西安郊区泾河大气成分站ρ(BC)(BC为黑碳)、粒子数浓度资料和观象台自动站、探空站数据,对西安郊区秋、冬季ρ(BC)变化特征、粒径分布特征和变化原因进行了分析.结果表明:①泾河郊区ρ(BC)比城区的低.城区ρ(BC)日变化呈三峰特征,峰值分别出现在凌晨02:00、清晨07:00和傍晚20:00,分别为17.0、12.5和21.5μgm3.泾河郊区ρ(BC)日变化呈双峰特征,峰值出现在上午09:00和晚上23:00,数值分别为5.5和6.1μgm3;谷值出现在清晨06:00和下午16:00,数值分别为4.9和2.6μgm3.②ρ(BC)与不同粒径颗粒物数浓度关系不同,其中与粒径〈4.0μm粒子的数浓度成正比,与粒径≥4.0μm粒子(如沙尘)的数浓度成反比;波长指数分析表明,沙尘可致ρ(BC)实测值偏大.③ρ(BC)与近地面逆温强度有密切相关性,R(相关系数)达到0.412 5(P〈0.000 1);风速小于1.5 ms时BC易堆积,大于1.5 ms时则相反;连续降水对BC清除效果显著.

英文摘要:

Black carbon (BC) is one of the most important research fields in aerosol climate effect studies due to its strong absorption effect. Compared to early international efforts, systematic BC observations were started late since 1990s' in several cities of China. The variation and particle size characteristics and their causing factors of BC concentration were analyzed based on data collected at Jinghe station, suburban of Xi' an, during autumn and winter (October 1st, 2008-February 28, 2009 ). The station is suitable for BC characteristics study since it is far from downtown area without main BC source nearby. The observational data included BC and particle concentration data collected by atmospheric elements station, meteorological variables collected by automatic meteorological station and sounding station. Results showed that: 1 ) suburban has lower BC concentration than urban area; Contrast to tri-peak diurnal cycle at urban area, suburban showed double-peak characteristic with maximum values of 5.5 p,g/m3 (09:00 o' clock) and 6. 1 p~g/m3 ( 23:00 o' clock). The two corresponding trough values were 4.9 p~g/m3 (06:00 o' clock) and 2. 6 p,g/m3 ( 16:00 o' clock) , respectively; 2 ) Relationship between BC concentration and particle size varied with particle sizes. The BC concentration was directly proportional to ultrafine particles and inversely proportional to big particles ( e. g. dust). Dust affects measurement of BC concentration; 3 ) BC concentration was significantly related with temperature inversion near the ground ( correlation coefficient). Wind speed had different effects in the processes of transport and diffusion of BC. Continuous precipitation had remarkable removal effects to BC. The increasing BC concentration during autumn could be contributed by the burning of crop stalks during the harvest seasons. In December and January, residential heating through burning coal and firewood by simple equipment caused relative high BC concentration. Th

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期刊信息
  • 《环境科学研究》
  • 中国科技核心期刊
  • 主管单位:中华人民共和国环境保护部
  • 主办单位:中国环境科学研究院
  • 主编:刘鸿亮
  • 地址:北京安外大羊坊8号中国环科院内
  • 邮编:100012
  • 邮箱:hjkxyj@163.com
  • 电话:010-84915128
  • 国际标准刊号:ISSN:1001-6929
  • 国内统一刊号:ISSN:11-1827/X
  • 邮发代号:82-384
  • 获奖情况:
  • 国内外数据库收录:
  • 俄罗斯文摘杂志,美国化学文摘(网络版),英国农业与生物科学研究中心文摘,波兰哥白尼索引,荷兰文摘与引文数据库,美国工程索引,美国剑桥科学文摘,英国动物学记录,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国国家哲学社会科学学术期刊数据库,中国北大核心期刊(2000版)
  • 被引量:33433