研究了Y0.75Ca0.25MnO3体系的结构和电磁特性,结果表明,场冷(FC)和零场冷(ZFC)直流磁化曲线在低温下存在典型的分叉现象,相应的Tcusp=34K;不同频率下交流磁化测量表明了随着频率的增加自旋冻结温度Tf=Tcusp向高温区移动,结合电输运测量,证明Y0.75Ca0.25MnO3体系为一典型的自旋玻璃绝缘(SGI)体系。
The structure and electromagnetic properties of perovskite manganite Y0.75 Ca0.25 MnO3 were systematically investigated. In low temperatures, a typical behavior of bifurcation was observed between field-cooled (FC) and zero-field-cooled (ZFC) magnetization with a cusp at Tcusp =34K in the ZFC magnetization curve. AC susceptibility also showed a cusp at Tf= Tcusp, called spin-glass freezing temperature, which shifts to high temperature with increasing frequencies. With the resistivity behavior in the electrical transport measurement, we considered an intrinsic spin-glass insulator (SGI) in the Y0.75 Ca0.25 MnO3 system.