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Ferrimagnetism and metal-insulator transition in an organic polymer chain
  • ISSN号:1674-1056
  • 期刊名称:《中国物理B:英文版》
  • 时间:0
  • 分类:O631.1[理学—高分子化学;理学—化学] TG146.36[金属学及工艺—金属材料;一般工业技术—材料科学与工程;金属学及工艺—金属学]
  • 作者机构:[1]Department of Physics, China Three Gorges University, Yichang 443002, China
  • 相关基金:Project supported by the National Natural Science Foundation of China (Grant Nos. 11204157 and 11174179), the China Three Gorges University Project (Grant No. KJ2011B068), and the Yichang City Project, China (Grant No. A201230229).
中文摘要:

The ferrimagnetism and quantum phase transition of a bipartite lozenge periodic Anderson-like organic polymer,in which the localized f electrons hybridize with the odd site conduction orbitals,are investigated by means of Green’s function theory.The ground state turns out to be gapless ferrimagnetism.At a finite temperature,the ferrimagnetic-toparamagnetic phase transition takes place.The Kondo screenings and Ruderman–Kittel–Kasuya–Yosida(RKKY)interaction can reduce and increase the transition temperature,respectively.Two Kondo screenings compete with each other,giving rise to the localized f electron spin screened antiferromagnetically.Accordingly,in a magnetic field,all spins are aligned along the chain easily,which is associated with metal–insulator transition.Furthermore,in a temperature-field plane,we reveal the gapless and spin polarized phases,which are characterized by susceptibility and specific heat,and whose behaviours are determined by the competition between the up-spin and down-spin hole excitations.

英文摘要:

The ferrimagnetism and quantum phase transition of a bipartite lozenge periodic Anderson-like organic polymer, in which the localized f electrons hybridize with the odd site conduction orbitals, are investigated by means of Green's function theory. The ground state turns out to be gapless ferrimagnetism. At a finite temperature, the ferrimagnetic-to- paramagnetic phase transition takes place. The Kondo screenings and Ruderman-Kittel-Kasuya-Yosida (RKKY) inter- action can reduce and increase the transition temperature, respectively. Two Kondo screenings compete with each other, giving rise to the localized f electron spin screened antiferromagnetically. Accordingly, in a magnetic field, all spins are aligned along the chain easily, which is associated with metal-insulator transition. Furthermore, in a temperature-field plane, we reveal the gapless and spin polarized phases, which are characterized by susceptibility and specific heat, and whose behaviours are determined by the competition between the up-spin and down-spin hole excitations.

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期刊信息
  • 《中国物理B:英文版》
  • 中国科技核心期刊
  • 主管单位:中国科学院
  • 主办单位:中国物理学会和中国科学院物理研究所
  • 主编:欧阳钟灿
  • 地址:北京 中关村 中国科学院物理研究所内
  • 邮编:100080
  • 邮箱:
  • 电话:010-82649026 82649519
  • 国际标准刊号:ISSN:1674-1056
  • 国内统一刊号:ISSN:11-5639/O4
  • 邮发代号:
  • 获奖情况:
  • 国内外数据库收录:
  • 被引量:406