利用飞秒时间分辨光抽运探测技术研究了电子型掺杂La2-xCexCuO4(LCCO)高温超导材料的准粒子超快动力学过程.得到低温(T〈0.7Tc)、转变温度附近(0.7Tc≤T≤Tc)和高温(T〉Tc)三个温区内的动力学行为.研究发现,低温时准粒子寿命随温度上升而下降,接近转变温度时出现反常的上升,正常态准粒子寿命受赝能隙影响明显大于金属中电声子的弛豫时间.还发现电子型掺杂LCCO光感生反射率变化AR/R动力学曲线存在皮秒量级的上升过程,它反映Cooper对被打散的时间较长,上升时间随温度增加而变短.采用Rothwad和Taylar提出的理论模型对实验结果进行了分析.
The quasiparticle dynamics in the electron-doped high-Tc superconductor La2- x Cex CuO4 (LCCO) was investigated by uhrafast time-resolved optical pump-probe technique. We present results in three temperature regions: namely the low temperature (T〈0.7Tc) region, that around Tc(0.7Tc≤ T≤ Tc) and the high temperature (T 〉 Tc) region. In general, there was a slowdown of the relaxation as the temperature decreases. However, the quasiparticle lifetime was found to exhibit a quasi-divergence as the temperature approached Te from below. The relaxation time in normal state was much longer than what was expected for metallic relaxation, indicating the presence of a T-independent pseudogap. We have also observed picosecond rise component of photoinduced change in reflectivity AR/R in the electron-doped LCCO, which is attributed to the Cooper pairbreaking dynamics. The rise time became shorter as the temperature increased. The experimental results are analyzed by Rothwarf-Taylor model.