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氮同位素控制下黄河及其主要支流硝酸盐来源分析
  • ISSN号:1673-4831
  • 期刊名称:生态与农村环境学报
  • 时间:2012
  • 页码:622-627
  • 分类:P342[天文地球—水文科学;天文地球—地球物理学] X522[环境科学与工程—环境工程]
  • 作者机构:[1]河南理工大学资源环境学院,河南焦作454000, [2]中国科学院地球化学研究所环境地球化学国家重点实验室,贵州贵阳550002, [3]济源市环境保护局沁园服务中心,河南济源454600
  • 相关基金:基金项目:国家自然科学基金(41103053);中国煤炭工业协会2010年度科学技术研究指导性计划项目(MTKJ2010-367)
  • 相关项目:南太行山山前平原地下水硫酸盐来源及迁移转化过程硫和氧同位素示踪研究
中文摘要:

选取黄河小浪底水库及以下干流和支流河水为主要研究对象,利用氮同位素识别河水潜在硝酸盐来源,结果表明,研究区黄河干流及支流沁河和伊洛河河水硝酸盐含量均值分别为(4.77±0.95)、(3.45±1.71)和(4.50±0.91)mg·L^-1研究区黄河干流河水δ15N-N03-均值为(+3.2±4.5)‰,上游河水硝酸盐来源主要为土壤有机氮矿化,下游平原区河水硝酸盐来源包括土壤有机氮矿化以及化学肥料。沁河河水δ15N—NO3-均值为(+8.3±4.6)‰,丰水期河水硝酸盐来源包括大气降水、土壤有机氮矿化以及化学肥料;平水期河水硝酸盐受到生活污水和土壤有机氮矿化共同影响;枯水期沁河河水由于断流形成封闭水体,浮游植物和藻类生长以及反硝化作用是控制河水硝酸盐的重要因素。枯水期洛河和伊河河水δ15N—NO3-值分别为+10.9‰和+3.4‰,其中生活污水是洛河河水硝酸盐的重要来源,合成化学肥料是伊河河水硝酸盐的重要来源。

英文摘要:

Human activities have greatly affected the nitrogen (N) cycles in the terrestrial and aquatic ecosystems. The Xiaolangdi Reservoir on the Yellow River and the mainstream and tributaries of the River thereafter, including Qin River and Yiluo River, were selected as subjects in this study to trace potential nitrate sources of the waters with nitrogen iso- tope. It was found that the average nitrate content in the mainstream of the Yellow Rvier and its tributaries, Qin River and Yiluo River, was (4. 77 ±0. 95) mg· L-1 , (3.45 ± 1.71 ) mg ·L-1 and (4. 50 ±0. 91 ) mg · L^-1 , respectively; and the average δ15N-NO3- in the mainstream was ( +3.2 ±4. 5)%0. Dissolved nitrate in upper stream of the Yellow River in the studied area came mainly from mineralized soil organic nitrogen, and in the rivers of the lower reaches from mineralized soil organic nitrogen and fertilizers applied. The average δ15 N-NO3- was ( + 8.3 ± 4. 6) %o in the Qin River. Its nitrate came mainly from atmospheric precipitation, mineralized soil organic nitrogen and fertilizers during the high water season, and from sewage water and mineralized soil organic nitrogen during the normal water season, and from growth of phyto- plankton and cyanobacteria, and denitrification in enclosed waters formed after the river discontiunued its flow during the low water season. Druing the low water season, the average 815N-NO~- was + 10. 9%o and + 3.4%0 in the Luo River and the Yi River respectively. In the former, sewage was the main source of nitrate, while in the latter the fertilizers. Key words : river; nitrate ; nitrogen isotope ; source identification ; Yellow River

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期刊信息
  • 《生态与农村环境学报》
  • 北大核心期刊(2011版)
  • 主管单位:中华人民共和国环境保护部
  • 主办单位:国家环境保护部南京环境科学研究所
  • 主编:蔡道基
  • 地址:江苏省南京市蒋王庙街8号
  • 邮编:210042
  • 邮箱:ere@vip.163.com
  • 电话:025-85287036
  • 国际标准刊号:ISSN:1673-4831
  • 国内统一刊号:ISSN:32-1766/X
  • 邮发代号:28-114
  • 获奖情况:
  • 全国优秀环境科技期刊,江苏省优秀期刊
  • 国内外数据库收录:
  • 美国化学文摘(网络版),英国农业与生物科学研究中心文摘,荷兰地学数据库,荷兰文摘与引文数据库,美国生物科学数据库,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版)
  • 被引量:7943