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Exploring the cooperation effect of DBD byproducts and Ag/TiO2 catalyst for water treatment in an APPJ system
  • ISSN号:1009-0630
  • 期刊名称:《等离子体科学与技术:英文版》
  • 时间:0
  • 分类:O53[理学—等离子体物理;理学—物理] X788.03[环境科学与工程—环境工程]
  • 作者机构:[1]Key Laboratory of Advanced Textile Materials and Manufacturing Technology and Engineering Research Center for Eco-Dyeing & Finishing of Textiles, Ministry of Education, Zhejiang Sci-Tech University,Hangzhou 310018, People's Republic of China, [2]Department of Chemistry and Chemical Engineering, University of New Haven, 300 Boston Post Road,West Haven, CT 06516, USA
  • 相关基金:the support from National Natural Science Foundation of China under Grant No.11175157; the Zhejiang Natural Science Foundations of China under No.LY16A050002; 521 Talent Project of Zhejiang Sci-Tech University; the Young Researchers Foundations of Zhejiang Provincial Top Key Academic Discipline of Chemical Engineering and Technology
中文摘要:

在这份报纸,把异构的 Ag/TiO 2 nanocomposite 催化剂与副产品相结合的集体效果(首先照耀和 O 3 种类) 一口气压血浆喷气(APPJ ) ,甲基橘子(瞬间) 的降级上的系统被探索。heterostructured Ag/TiO 2 nanocomposite 经由通过一个热水的方法在商业地可得到的 TiO 2 催化剂(P25 ) 上装饰 Ag 量点(QD ) 被完成。nanocomposite 催化剂的 X 光衍射分析在 44.3m 揜?揜 显示出衍射山峰吗??

英文摘要:

In this paper,the collective effects of combining heterogeneous Ag/TiO2 nanocomposite catalyst with the byproducts(primarily the irradiation and the O3 species) of an atmospheric pressure plasma jet(APPJ) system on the degradation of methyl orange(MO) were explored.The heterostructured Ag/TiO2 nanocomposite was achieved via decorating the Ag quantum dots(QDs) on the commercially available TiO_2catalyst(P25) through a hydrothermal method.The x-ray diffraction analysis of the nanocomposite catalyst showed the diffraction peaks at 44.3°,64.4°,and 77.5°,corresponding to the Ag planes of(200),(220) and(311),respectively.The high resolution transmission electron microscope characterization of the nanocomposite catalyst indicated that the Ag QDs with an average diameter of 5 nm were homogeneously distributed on the P25 surface.The experimental results on the MO photodegradation showed that the APPJ irradiation had a marginal effect on the cleavage of the MO molecules.When the Ag/TiO2 nanocomposite catalyst was used,the photodegradation rate of MO increased about 5 times.When both the APPJ byproducts and the Ag/TiO2 nanocomposite catalyst were used,however,over 90% of the MO in the tested solution was cleaved within 15 min,and the energy efficiency was about 0.6 g/k W h.Moreover,an optimal Ag dosage value was determined(6 wt%).The catalytic results indicated that combining the DBD plasma byproducts with heterogeneous nanocomposite catalysts may be an effect protocol for decreasing the application cost of the DBD system and mitigating the environment pollution by organic dyes in the textile industry.

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期刊信息
  • 《等离子体科学与技术:英文版》
  • 主管单位:中国科学院 中国科协
  • 主办单位:中国科学院等离子体物理研究所 中国力学学会
  • 主编:万元熙、谢纪康
  • 地址:合肥市1126信箱
  • 邮编:230031
  • 邮箱:pst@ipp.ac.cn
  • 电话:0551-5591617 5591388
  • 国际标准刊号:ISSN:1009-0630
  • 国内统一刊号:ISSN:34-1187/TL
  • 邮发代号:
  • 获奖情况:
  • 国内外数据库收录:
  • 美国化学文摘(网络版),荷兰文摘与引文数据库,美国工程索引,美国剑桥科学文摘,美国科学引文索引(扩展库),英国科学文摘数据库
  • 被引量:89