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常规处理工艺对饮水中MX及致突变性影响
  • ISSN号:1001-0580
  • 期刊名称:中国公共卫生
  • 时间:0
  • 页码:782-784
  • 语言:中文
  • 分类:R123.6[医药卫生—环境卫生学;医药卫生—公共卫生与预防医学] R994.6[医药卫生—毒理学;医药卫生—药学]
  • 作者机构:[1]华中科技大学同济医学院公共卫生学院劳动卫生与环境卫生学系、教育部环境与健康重点实验室,武汉430030, [2]湖北省武汉市水务集团有限公司水质监测中心, [3]湖北省武汉市东西湖自来水公司
  • 相关基金:国家自然科学基金(20577012)
  • 相关项目:氯化消毒副产物MX形成影响因素及其健康效应研究
中文摘要:

目的研究3-氯-4-二氯甲基-5-羟基-2(5氢)-呋喃酮(MX)和总有机碳(TOC)浓度以及非挥发性有机提取物致突变性在饮用水常规处理工艺过程中的变化,为城市给水处理工艺优化提供依据。方法采集某自来水厂饮用水常规处理工艺过程中的源水、预加氯后的混凝沉淀水、沉淀水、过滤水、加氯消毒后的出厂水和管网末梢水。采用气相色谱/质谱联用(GC/MS)和TOC分析仪分别检测水样MX浓度和TOC浓度,Ames试验检测水样非挥发性有机提取物的致突变性,同时检测水样的浊度和pH值。结果常规处理工艺过程中不同工艺段水样MX和TOC浓度的变化趋势一致,与源水比较,均表现为预加氯和加氯消毒后二者浓度上升,经过沉淀处理后二者浓度下降;水中MX的生成量与TOC浓度呈显著正相关,而与水的浊度和pH值无相关关系;加氯消毒后的出厂水和管网末梢水致突变活性也有所增加。结论在饮用水常规处理工艺过程中,加氯和沉淀工艺是影响MX和TOC浓度的重要环节;加氯可增加饮用水中MX的生成量和致突变活性,影响饮水安全。

英文摘要:

Objective To study the effect of routine water treatment technology on contents of 3-cloro-4- (dichloromethyl)-5-hydroxy-2(SH)-furanone(MX) and total organic carbon(TOC) in drinking water, as well as mutagenicity of the non-volatile organic extracts from drinking water for providing scientific bases for optimization of the drinking water treatment technology. Methods Water samples including raw water, water from treatment steps of coagulative precipitation after prechlorination, precipitation, filtration and chlorination disinfection, and tap water were collected. GC/MS and TOC- Analyse were used to determine the concentrations of MX and TOC. The pH value and turbidity of water were also determined. The mutagenicity of non-volatile organic extracts from water samples was evaluated by means of Ames test. Results MX and TOC concentrations showed the same variation during the process of drinking water treatment. Compared to raw water, MX and TOC levels in water were increased after prechlorination and chlorination disinfection and decreased after precipitation. MX levels were signinficantly correlated with TOC levels, but not with pH value and turbidity. There were higher mutagenic activities of water after chlorination disinfection and tap water than that of raw water. Conclusion For drinking water treatment technology, chlorination and precipitation were important procedures affecting concentrations of MX and TOC. Chlorination enhances formation of MX and mutagenic activity of drinking water.

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期刊信息
  • 《中国公共卫生》
  • 北大核心期刊(2011版)
  • 主管单位:国家卫生和计划生育委员会
  • 主办单位:中华预防医学会
  • 主编:王宇
  • 地址:沈阳市和平区砂阳路242号
  • 邮编:110005
  • 邮箱:zgggws@vip.sina.com
  • 电话:024-23388443 23388479
  • 国际标准刊号:ISSN:1001-0580
  • 国内统一刊号:ISSN:21-1234/R
  • 邮发代号:8-204
  • 获奖情况:
  • 1999年获中华预防医学会系列期刊优秀期刊二等奖,2000年获中华预防医学会系列期刊优秀期刊三等奖,国家期刊提名奖
  • 国内外数据库收录:
  • 美国化学文摘(网络版),中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国北大核心期刊(2000版)
  • 被引量:66800