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Seasonal variations of sulfur aerosols at Zhongshan Station, East Antarctica
  • 分类:P728.2[天文地球—海洋科学] X703[环境科学与工程—环境工程]
  • 作者机构:[1]Key Laboratory of Global change and Marine-Atmospheric Chemistry, SOA, Third Institute of Oceanography, StateOceanic Administration, Xiamen 361005, China
  • 相关基金:Acknowledgments Many thanks go to the staff of Zhongshan Station for supporting the field operation, and to Mr. Guoqiang Qiu from Xiamen University for providing remote sensor method assistance. This work was supported by the National Natural Science Foundation of China (NSFC) (Grant nos. 41476172, 41230529, 40671062, and 41106168), the Chinese Polar Environment Comprehensive Investigation & Assessment Programs (Grant no. CHINARE2012-15 for 01-04-02, 02-01, and 03-04- 02), and International Cooperation Programs, Chinese Arctic and Antarctic Adminstration (Grant nos. 2G22010, IC201201, IC201308, and IC201513).
中文摘要:

Observations of atmospheric methane-sulfonic acid(MSA) and non-sea-salt sulfate(nss-SO42-) from December 2010 to November 2011 at Zhongshan Station are presented in this paper. MSA and nss-SO42- average concentrations were 24.2 ± 37.9 ng·m-3(0.5–158.3 ng·m-3) and 53.0 ± 82.6 ng·m-3(not detected [n.d.]) – 395.4 ng·m-3), respectively. Strong seasonal variations of MSA and nss-SO42-, with maxima in austral summer and minima in winter, were examined. The high concentrations of sulfur compounds in December may be attributed the dimethyl sulfide(DMS) emissions from the marginal ice zone, when open water near the sampling site was important in impacting the sulfur species of January and February at Zhongshan Station. In austral winter, there was almost no phytoplanktonic activity in offshore waters, and atmospheric sulfur compounds likely had long-range transport sources.

英文摘要:

Observations of atmospheric methane-sulfonic acid(MSA) and non-sea-salt sulfate(nss-SO4^2-) from December 2010 to November 2011 at Zhongshan Station are presented in this paper. MSA and nss-SO4^2- average concentrations were 24.2 ± 37.9 ng·m^-3(0.5-158.3 ng·m^-3) and 53.0 ± 82.6 ng·m^-3(not detected [n.d.]) - 395.4 ng·m^-3), respectively. Strong seasonal variations of MSA and nss-SO4^2-, with maxima in austral summer and minima in winter, were examined. The high concentrations of sulfur compounds in December may be attributed the dimethyl sulfide(DMS) emissions from the marginal ice zone, when open water near the sampling site was important in impacting the sulfur species of January and February at Zhongshan Station. In austral winter, there was almost no phytoplanktonic activity in offshore waters, and atmospheric sulfur compounds likely had long-range transport sources.

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