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激光诱导等离子体对水OH伸缩振动受激拉曼散射的影响
  • ISSN号：1000-3290
  • 期刊名称：《物理学报》
  • 时间：0
  • 分类：O53[理学—等离子体物理;理学—物理]
  • 作者机构：[1]吉林大学物理学院,长春130012
  • 相关基金：国家自然科学基金（批准号：11104106,11374123）、国家基础科学人才培养基金（批准号：J1103202）、吉林省科技厅项目（批准号：201101037,201201030,20130101017JC,20140101173JC,20140204077GX）和中国博士后科学基金（批准号：2012M520669,2013M530973）资助的课题.
作者： 汪胜晗, 李占龙[1], 孙成林[1], 里佐威[1], 门志伟[1]
关键词： 受激拉曼散射, 激光诱导等离子体, 氢键, 水分子, stimulated Raman scattering, laser-induced plasma generation, hydrogen bonds, water molecules
中文摘要：

利用532nm脉冲激光进行水的受激拉曼散射研究，通过改变激光焦点与水一空气界面的距离，获得截然不同的0H伸缩振动受激斯托克斯和反斯托克斯谱线．焦点距水一空气界面大于20mm时，只存在＋3400cm-1的斯托克斯和反斯托克斯谱线；焦点距离水．空气界面小于20mm时，存在±3000和±3400cm-1的斯托克斯和反斯托克斯谱线；继续缩小焦点与水一空气界面的距离，3000cm-1谱线被增强，而3400cm-1谱线被削弱．研究结果表明，激光诱导水产生的等离子体增强了局部水分子的氢键，导致0H伸缩振动红移，同时过剩电子增强了水的OH伸缩振动受激拉曼散射．

英文摘要：

532 nm pulse beam is used to induce the stimulated Raman scatting of water molecules. Different Stocks and anti- Stocks characteristic peaks of OH stretching vibrational from water molecules are obtained when the position of the focal spot is changed. The unique ~3400 cm-I Stokes characteristic peak with its anti-Stokes is present when the distance between focal spot and interface is fixed to be over 20 mm; both ~：3000 cm-I and ：1：3400 cm-1 with their anti-Stokes exist when the distance is reduced under 20 ram; both characteristic peaks are enhanced especially the 3000 cm-I peak whose change is more remarkable when the spot continues to move up. Experimental results indicate that laser-induced plasma generated from water molecules enhances the stimulated Raman scattering of OH stretching vibrational from water molecules by affecting hydrogen bonds between water molecules and OH from single water molecules.

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期刊信息
  • 《物理学报》
  • 北大核心期刊（2011版）
  • 主管单位:中国科学院
  • 主办单位:中国物理学会 中国科学院物理研究所
  • 主编：欧阳钟灿
  • 地址：北京603信箱(中国科学院物理研究所)
  • 邮编：100190
  • 邮箱：apsoffice@iphy.ac.cn
  • 电话：010-82649026
  • 国际标准刊号：ISSN：1000-3290
  • 国内统一刊号：ISSN：11-1958/O4
  • 邮发代号:2-425
  • 获奖情况:
  • 1999年首届国家期刊奖,2000年中科院优秀期刊特等奖,2001年科技期刊最高方阵队双高期刊居中国期刊第12位
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  • 被引量:49876