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Iodine speciation in aerosol particle samples collected over the sea between offshore China and the Arctic Ocean
  • 分类:P731.15[天文地球—海洋科学] U453[建筑科学—桥梁与隧道工程;交通运输工程—道路与铁道工程]
  • 作者机构:[1]Institute of Polar Environment, University of Science and Technology of China, Hefei 230026, China, [2]Chinese Academy of Meteorological Sciences, Beijing 100081, China
  • 相关基金:Acknowledgments This work was supported by the Chinese Polar Environment Comprehensive Investigation & Assessment Programs (Grant no. CHINARE 2011-2015), the National Natural Science Foundation of China (Grant no. 41176170). We thank the NOAA Air Resources Laboratory (ARL) for making the HYSPLIT transport and dispersion model available on the Internet (http://www.arl.noaa.gov/ready.html).
中文摘要:

The concentrations of carbon monoxide and ozone in the marine boundary layer were measured during the 6th Chinese National Arctic Research Expedition(from July to September, 2014). Carbon monoxide concentration ranged between 47.00 and 528.52 ppbv with an average of 103.59 ± 40.37 ppbv. A slight decrease with increasing latitude was observed, except for the extremely high values over the East China Sea which may be attributed to anthropogenic emissions. Ozone concentration ranged between 3.27 and 77.82 ppbv with an average of 29.46±10.48 ppbv. Ozone concentration decreased sharply with increasing latitude outside the Arctic Ocean(during both the northward and the southward course), while no significant variation was observed over the Arctic Ocean. The positive correlation between carbon monoxide and ozone in most sections suggests that the ozone in the marine boundary layer mainly originated from photochemical reactions involving carbon monoxide.

英文摘要:

The concentrations of carbon monoxide and ozone in the marine boundary layer were measured during the 6th Chinese National Arctic Research Expedition(from July to September, 2014). Carbon monoxide concentration ranged between 47.00 and 528.52 ppbv with an average of 103.59 ± 40.37 ppbv. A slight decrease with increasing latitude was observed, except for the extremely high values over the East China Sea which may be attributed to anthropogenic emissions. Ozone concentration ranged between 3.27 and 77.82 ppbv with an average of 29.46±10.48 ppbv. Ozone concentration decreased sharply with increasing latitude outside the Arctic Ocean(during both the northward and the southward course), while no significant variation was observed over the Arctic Ocean. The positive correlation between carbon monoxide and ozone in most sections suggests that the ozone in the marine boundary layer mainly originated from photochemical reactions involving carbon monoxide.

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