研究了三种掺Yb钒酸盐混晶Yb0.005:Y0.298Gd0.697VO4,Yb0.007:Y0.407Gd0.586VO4和Yb0.009:Y0.575Gd0.416VO4的室温偏振吸收谱和发射谱.结果表明,最强的吸收和发射相应于π偏振,位于波长985nm;随组分不同,最大吸收截面σabs=4.8—8.5×10-20cm2,吸收带宽9.5—9.9nm;最大受激发射截面σem=5.8—10.3×10-20cm2.利用高亮度半导体激光器纵向抽运实现了室温下的连续波激光运转.研究发现,不同混晶的激光振荡行为存在很大差异:在谐振腔输出耦合透过率T=2%条件下,Yb0.005:Y0.298Gd0.697VO4和Yb0.009:Y0.575Gd0.416VO4的激光振荡随抽运功率降低而出现σ,π偏振态的共存和转变;而Yb0.007:Y0.407Gd0.586VO4的激光振荡则保持π偏振态不变.在T=5%情形,Yb0.009:Y0.575Gd0.416VO4的激光振荡为单纯的σ偏振;而Yb0.005:Y0.298Gd0.697VO4所产生的激光振荡随抽运功率下降仍出现类似的偏振态变化行为.
The room-temperature polarized absorption and emission spectra of Yb doped mixed vanadates Yb0.005:Y0.298 Gd0.697 VO4,Yb0.007:Y0.407 Gd0.586 VO4,and Yb0.009: Y0.575 Gd0.416 VO4 have been studied. The results show that the strongest absorption and emission,occurring at wavelength of 985 nm,correspond to the π polarization,depending on the composition the maximum absorption cross section ranges from 4. 8 to 8. 5 × 10-20 cm2,with bandwidths of 9. 5—9. 9 nm, whereas the maximum stimulated emission cross section varies in the range of 5. 8—10. 3 × 10-20 cm2. Continuous-wave laser operation has been realized at room temperature with the mixed crystals through longitudinal pumping with a diode laser. It was found that the laser oscillation behavior differs significantly from one mixed crystal to another:in the case of T = 2% ( T is the output coupling of the resonator),the coexistence and switching of σ,π polarization states occur on reducing the pump power in the laser oscillation of Yb0.005:Y0.298 Gd0.697 VO4 and Yb0.009:Y0.575 Gd0.416 VO4,while the laser oscillation of Yb0.007:Y0.407Gd0.586VO4 is capable of maintaining its π polarization state. In the case of T = 5% ,however, the laser oscillation generated with Yb0.009:Y0.575 Gd0.416 VO4 is purely σ-polarized,whereas the laser behavior of Yb0.005: Y0.298Gd0.697VO4 is similar to that exhibited in the case of T=2% .