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中文摘要：
项目执行期间，制备和研究了系列具有磁性孔洞的氨基酸-稀土-过渡金属簇,尤其是在风扇形分子研究方面取得了有影响的结果；研究了具有多孔结构的硫属、唑类或胺类高聚物和具有各种维数结构的新型有机膦酸盐材料，在热致或光致变色的化合物机理研究方面取得了重要进展；合成出倍频系数是目前所报道的硼酸盐材料体系中最大值的碘硼酸铅化合物，同时制备出具有良好倍频效应以及在中红外非线性光学材料方面具有潜在应用前景的系列稀土锑硫化物；探索出窄带半导体热电化合物新体系，合成了首例锑基笼合物，实现了笼状化合物的结构调控；发现了双隧道Te基化合物，在热电化合物的研究方面取得了一定进展；发现了利用碱金属或碱土金属为模板合成无心或手性空间群配位聚合物晶体的新方法，得到了若干具有KDP 2-5倍的二阶非线性光学性能和铁电性能的金属/羧酸体系；合成了系列唯铁氢化酶的模型化合物，并较系统和深入地研究了其结构与催化产氢活性；同时研究了系列含硫仿生团簇的多种结构的组装，并在光催化方面取得了一定的进展；欧洲Springer出版了吴新涛院士主编的对一些无机体系的控制组装进行了系统总结的英文专著。
结论摘要：
英文主题词Cluster ccompounds; Controlled assembly; Structural modification; Properties；Functional materials
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期刊论文
Syntheses, topological analyses, and NLO-active properties of new Cd(II)/M(II) (M = Ca, Sr) metal-or
Cluster-Based Cu(II)-Azide Polymers: Synthesis, Structure, Magnetic Properties, and Effect of Polyam
Synthesis, Crystal and Electronic Structures, and Physical Properties of Caged Ternary Cu-Rich Antim
Structural Characteristics, Electronic Structure, and Thermoelectric Property of New Sb-Based Type-I
A Series of Cation-Templated, Polycarboxylate-Based Cd(II) or Cd(II)/Li(I) Frameworks with Second-Or
A series of novel Pb(II) or Pb(II)/M(II) (M = Ca and Sr) hybrid inorganic-organic frameworks based o
Synthesis, structures and luminescent properties of new Pb(II)/M(I) (M= K, Rb and Cs) frameworks bas
Structure Change Induced by Terminal Sulfur in Noncentrosymmetric La2Ga2GeS8 and Eu2Ga2GeS7 and Nonl
Contribution of Disulfide S(2)(2-) Anions to the Crystal and Electronic Structures in Ternary Sulfid
Syntheses, Structures, and Magnetic and Thermoelectric Properties of Double-Tunnel Tellurides: A(x)R
Syntheses, Structure, Physical Properties, and Electronic Structures of DyCu(x)Al(12-x) (4.0 <= x <=
A new cumulene diiron complex related to the active site of Fe-only hydrogenases and its phosphine s
Two new ferrimagnetic Mn(II)-carboxylate coordination polymers constructed from 5-tert-butyl isophth
Synthesis, structures and physical properties of new 3D lanthanide coordination polymers constructed
Lanthanide metal organic frameworks based on octahedral secondary building units: Structural, lumine
Three New d(10) Coordination Polymers with Arenedisulfonates: Syntheses, Crystal Structures and Lumi
Syntheses, crystal structures, thermal stabilities, luminescence and magnetism of two 3D pillared me
Syntheses, topological analyses and magnetic properties of two 3D supramolecular nickel-organic fram
Syntheses, topological analyses and photoelectric properties of Ag(I)/Cu(I) metal-organic frameworks
Assembly of Novel 2D and 3D Heterometallic Sb(III)-Cu(I) Polymers Based on Antimony(III) Thiolates a
Synthesis, Properties, and Theoretical Studies of New Stepwise Layered Iodoplumbate: [Ni(opd)(2)(acn
Syntheses, Structures, and Theoretical Studies of New Ternary Antimonides beta-RECoSb(3) (RE = La-Nd
Structural Diversity of Infinite 3d-4f Heterometallic Cluster Compounds Driven by Various Lanthanide
Syntheses, Crystal and Electronic Structures, and Physical Properties of Two Quaternary Chalcogenide
Synthesis, topology analysis and luminescent property of a 3D AgCN coordination polymer based on 2-t
Syntheses and Characterization of Two Novel Mo(W)/Cu/S Dodecanuclear Clusters with Triple Incomplete
Can the Localization Regime of [GaNNW/BNNT] Nanocables Change from Type II to Type I? First-Principl
Syntheses, topological structures and physical properties of two 2D lanthanide-organic frameworks co
Submicrosized Rods, Cables, and Tubes of ZnE (E = S, Se, Te): Exterior-Interior Boron-Chalcogen Conv
Four W(Mo)/Cu/S complexes containing N-heterocyclic thiones as linkers: Synthesis, structures and op
Syntheses, characterizations and topology analyses of two 3D copper-organic frameworks from Cu(pyzca
Structures and Physical Properties of Rare-Earth Zinc Antimonides Pr(6)Zn(1+x)Sb(14+y) and RE(6)Zn(1
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