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Influence of Ionization Degrees on Conversion of CO and CO2 in Atmospheric Plasma near the Ground
  • ISSN号:1009-0630
  • 期刊名称:《等离子体科学与技术:英文版》
  • 时间:0
  • 分类:O646.1[理学—物理化学;理学—化学] TM862[电气工程—高电压与绝缘技术]
  • 作者机构:[1]College of Physics Science and Technology, Hebei University,Hebei Key Lab of Optic-electronic Information and Materials, Baoding 071002, China
  • 相关基金:supported by the Research Foundation of Education Bureau of Hebei Province, China (No. Q2012084), National Natural Science Foundation of China (No. 10805013) and Natural Science Foundation of Hebei Province, China (No. A2011201132)
中文摘要:

A zero-dimensional model is used to study the processes of physical and chemical reactions in atmospheric plasma with different ionization degrees near the ground(0 km). The temporal evolutions of CO, CO2and other main reactants(namely OH and O2), which affect the conversion of CO and CO2, are obtained for afterglow plasma with different initial values. The results show that the consumption rate of CO is largest when the initial electron number density ne0=1012cm-3, i.e. the ionization degree is 0.000004%. The number density of CO2is relatively small when ne0=1016cm-3, i.e. the ionization degree is 0.04%, whereas they are very close under the condition of other ionization degrees. Considering the total number densities of CO and CO2and the consumption rate of CO comprehensively, the best condition is ne0=1013cm-3, i.e. the ionization degree is 0.00004% for reducing the densities of CO and CO2in the atmospheric plasma.The temporal evolutions of N+, Ar+, CO+and CO+2are also shown, and the influences on the temporal evolutions of CO and CO2are analyzed with increasing ionization degree.

英文摘要:

A zero-dimensional model is used to study the processes of physical and chemical reactions in atmospheric plasma with different ionization degrees near the ground (0 km). The temporal evolutions of CO, C02 and other main reactants (namely OH and O2), which affect the conversion of CO and C02, are obtained for afterglow plasma with different initial values. The results show that the consumption rate of CO is largest when the initiM electron number density neo=1012 cm-3, i.e. the ionization degree is 0.000004%. The number density of CO2 is relatively small when neo=1016 cm-3, i.e. the ionization degree is 0.04%, whereas they are very close under the condition of other ionization degrees. Considering the total number densities of CO and C02 and the consumption rate of CO comprehensively, the best condition is neo=1013 cm-3, i.e. the ionization degree is 0.00004% for reducing the densities of CO and CO2 in the atmospheric plasma. The temporal evolutions of N+, Ar+, CO+ and CO+ are also shown, and the influences on the temporal evolutions of CO and C02 are analyzed with increasing ionization degree.

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期刊信息
  • 《等离子体科学与技术:英文版》
  • 主管单位:中国科学院 中国科协
  • 主办单位:中国科学院等离子体物理研究所 中国力学学会
  • 主编:万元熙、谢纪康
  • 地址:合肥市1126信箱
  • 邮编:230031
  • 邮箱:pst@ipp.ac.cn
  • 电话:0551-5591617 5591388
  • 国际标准刊号:ISSN:1009-0630
  • 国内统一刊号:ISSN:34-1187/TL
  • 邮发代号:
  • 获奖情况:
  • 国内外数据库收录:
  • 美国化学文摘(网络版),荷兰文摘与引文数据库,美国工程索引,美国剑桥科学文摘,美国科学引文索引(扩展库),英国科学文摘数据库
  • 被引量:89