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Cesium lead halide perovskite triangular nanorods as high-gain medium and effective cavities for multiphoton- pumped lasing
  • ISSN号:2095-0462
  • 期刊名称:《物理学前沿:英文版》
  • 时间:0
  • 分类:O484.1[理学—固体物理;理学—物理] TN929.11[电子电信—通信与信息系统;电子电信—信息与通信工程]
  • 作者机构:[1]School of Physics and Electronics, Key Laboratory for Micro-Nano Physics and Technology of Hunan Province, and State Key Laboratory of Chemo/Biosensing and Chemometrics, Hunan University, Changsha 410082, China, [2]Institute of Physical and Theoretical Chemistry, University of Tübingen, Aufder Morgenstelle 18, 72076 Tübingen, Germany
  • 相关基金:Acknowledgements All authors are grateful to the National Natural Science Foundation of China (Nos. 51525202, 61574054, 61505051 and 61474040), the Hunan province science and technology plan (Nos. 2014FJ2001 and 2014TT1004), the Aid program for Science and Technology Innovative Research Team in Higher Educational Institutions of Hunan Province, and the Fundamental Research Funds for the Central Universities.
中文摘要:

基于铯铅卤化物 perovskite, nanostructures 在综合 photonics 为非线性的光学和实际频率 upconversion 设备正在答应的高效的抽 multiphoton 的激光。然而,如此的激光的表演高度依赖于材料和洞的质量,它使他们的制造挑战性。此处,我们表明经由蒸汽方法制作的三角形的 nanorods 能作为抽 multiphoton 的激光的获得媒介和有效的洞服务的那铯铅卤化物 perovskite。我们观察了在刺激的放射激光的模式蓝移动在增加的刺激的 fluence 依赖的放射激光系列驱动充满效果的乐队引起的移动,它与 Burstein 苔藓的动力学适合很好。而且,在 CsPbBr 3 nanorods 放射激光的有效 multiphoton 能在一个宽刺激波长范围(700-1,400 nm ) 被认识到。放射激光的 multiphoton 的动力学被解决时间的光致发光光谱学调查,它显示电子洞血浆负责抽 multiphoton 的放射激光。这个工作能在放射激光的频率 upconversion 为铯铅卤化物 perovskite nanostructures 导致新机会和应用设备并且光互连系统。

英文摘要:

High-performance multiphoton-pumped lasers based on cesium lead halide perovskite nanostructures are promising for nonlinear optics and practical frequency upconversion devices in integrated photonics. However, the performance of such lasers is highly dependent on the quality of the material and cavity, which makes their fabrication challenging. Herein, we demonstrate that cesium lead halide perovskite triangular nanorods fabricated via vapor methods can serve as gain media and effective cavities for multiphoton-pumped lasers. We observed blue-shifts of the lasing modes in the excitation fluence-dependent lasing spectra at increased excitation powers, which fits well with the dynamics of Burstein-Moss shifts caused by the band filling effect. Moreover, efficient multiphoton lasing in CsPbBr3 nanorods can be realized in a wide excitation wavelength range (700-1,400 nm). The dynamics of multiphoton lasing were investigated by time-resolved photoluminescence spectroscopy, which indicated that an electron-hole plasma is responsible for the multiphoton-pumped lasing. This work could lead to new opportunities and applications for cesium lead halide perovskite nanostructures in frequency upconversion lasing devices and optical interconnect systems.

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期刊信息
  • 《物理学前沿:英文版》
  • 主管单位:中华人民共和国教育部
  • 主办单位:高等教育出版社
  • 主编:赵光达
  • 地址:北京市朝阳区惠新东街4号富盛大厦15层
  • 邮编:100029
  • 邮箱:
  • 电话:
  • 国际标准刊号:ISSN:2095-0462
  • 国内统一刊号:ISSN:11-5994/O4
  • 邮发代号:80-965
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  • 被引量:3