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MoTe2 is a good match for Gel by preserving quantum spin Hall phase
  • ISSN号:1000-6818
  • 期刊名称:《物理化学学报》
  • 时间:0
  • 分类:O[理学]
  • 作者机构:[1]School of Physics, Shandong University, Jinan 250100, China, [2]State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China, [3]Peter Grunberg Institut and Institute for Advanced Simulation, Forschungszentrum JOlich and JARA, 52425 Julich, Germany, [4]Department of Physics and Earth Sciences, Jacobs University Bremen, Campus Ring 1, 28759 Bremen, Germany
  • 相关基金:This work is supported by the National Basic Research Program of China (No. 2013CB632401), National Natural Science Foundation of China (Nos. 21333006, 11374190, and 1140418), and Program of Introducing Talents of Discipline to Universities (111 Program) (No. 297B13029). We also thank the Taishan Scholar Program of Shandong Province.
中文摘要:

量旋转霍尔(QSH ) 绝缘体是快速在压缩事的物理正在变得主流的材料的一个新班。为 QSH 绝缘体的发展的主要障碍是他们和底层的强壮的相互作用使他们困难试验性地学习。在这研究,使用密度功能的理论,我们发现尘埃 2 是为 GeI 单层的一根好火柴。货车 der Waals GeI/MoTe 2 heterosheet 的热稳定性经由分子动力学的模拟被检验。扫描通道显微镜学模仿表明 GeI 单层完美地保存尘埃 2 的 bulked 蜂房结构。尘埃 2 上的 GeI 被证实由直接计算旋转 Chern 数字是 1 与 0.24 eV 的相当大的间接体积 bandgap 维持它的拓扑的乐队结构。是期望, GeI 的电子活动性被尘埃 2 提高底层限制。根据有有效团的近似的变丑潜力理论, GeI/MoTe 2 的电子活动性作为 372.7 厘米 2  被估计吗??

英文摘要:

Quantum spin Hall (QSH) insulator is a new class of materials that is quickly becoming mainstream in condensed-matter physics. The main obstacle for the development of QSH insulators is that their strong interactions with substrates make them difficult to study experimentally. In this study, using density functional theory, we discovered that MoTe2 is a good match for a GeI monolayer. The thermal stability of a van der Waals GeI/MoTe2 heterosheet was examined via molecular-dynamics simulations. Simulated scanning tunneling microscopy revealed that the GeI monolayer perfectly preserves the bulked honeycomb structure of MoTe2. The GeI on MoTe2 was confirmed to maintain its topological band structure with a sizable indirect bulk bandgap of 0.24 eV by directly calculating the spin Chern number to be -1. As expected, the electron mobility of the GeI is enhanced by MoTe2 substrate restriction. According to deformation- potential theory with the effective-mass approximation, the electron mobility of GeI/MoTe2 was estimated as 372.7 cm^2·s^-1·V^-1 at 300 K, which is 20 times higher than that of freestanding GeI. Our research shows that traditional substrates always destroy the topological states and hinder the electron transport in QSH insulators, and pave way for the further realization and utilization of QSH insulators at room temperature.

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期刊信息
  • 《物理化学学报》
  • 中国科技核心期刊
  • 主管单位:中国科学技术协会
  • 主办单位:北京大学化学与分子工程学院承办
  • 主编:刘忠范
  • 地址:北京大学化学楼
  • 邮编:100871
  • 邮箱:whxb@pku.edu.cn
  • 电话:010-62751724
  • 国际标准刊号:ISSN:1000-6818
  • 国内统一刊号:ISSN:11-1892/O6
  • 邮发代号:82-163
  • 获奖情况:
  • 中文核心期刊
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  • 俄罗斯文摘杂志,美国化学文摘(网络版),荷兰文摘与引文数据库,美国科学引文索引(扩展库),英国科学文摘数据库,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),英国英国皇家化学学会文摘,中国北大核心期刊(2000版)
  • 被引量:24781