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中文摘要：
本项目以炭(C)基半导体复合光催化剂可有效提高有机物污染物降解效率的实验事实为指导，拟设计合成一系列C/半导体光催化剂纳米晶（ZnO、ZnS、CdS、TiO2）复合材料从单分散的C/半导体纳米晶核壳结构复合球的可控合成和光催化性能研究到外加磁场诱导一维Fe3O4/C/半导体纳米晶三明治结构的复合材料自组装，实现其高效循环使用功能；从ZnO/C/半导体纳米晶三明治结构纳米棒的可控制备及其所构建的光催化协同反应场作用机制的研究到ZnO（TiO2）/C/半导体纳米晶复合纳米棒（管）在基片上阵列生长，实现其由介观到宏观的光催化剂器件化。项目的研究结果不仅有助于探索不同类型的炭基半导体纳米复合材料的可控合成方法，揭示其提高光催化降解活性的一般规律，促进此类复合光催化材料从理论到应用跨越的研究。同时，也为推动其工业化应用提供一定的技术储备和保障。
英文摘要：
C-based semiconductors；nanocrystalsemiconductor photocatalysts；controllable preparation；photocatalytic degradation；
结论摘要：
本项目已完成了各项研究内容，实现预期的成果。已设计合成新型高效的炭（C）基半导体（CdS、ZnS、ZnO、TiO2）纳米晶复合光催化剂。通过对单分散的C/半导体纳米晶核壳结构的控制合成、宏量制备、结构与光催化性能关系的研究，设计在外加磁场诱导下自组装形成单分散的Fe3O4 /C/半导体纳米晶一维有序链状三明治结构的复合光催化剂。成功实现了对ZnO/C/半导体纳米晶三明治结构的可控合成。在上述工作的基础上，本项目研究人员成功制备出一系列Ag-基Bi-基半导体纳米复合材料。本项目的成功实施，不仅可以为新型炭/半导体纳米复合结构材料的可控制备提供新的设计思想，而且为污水处理技术的发展提供一系列新型光催化剂。在基金支持下发表SCI论文33篇, 其中一区及二区TOP论文24篇，3篇论文被ESI选为高被引论文，获授权发明专利4项，获浙江省自然科学二等奖1项。
成果综合统计
期刊论文
会议论文
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期刊论文
Microwave-Assisted Synthesis of Porous Ag2S–Ag Hybrid Nanotubes with High Visible-Light Photocatalyt
Facile one-step microwave-assisted route towards Ni nanospheres/reduced graphene oxide hybrids for n
Assembling carbon-coated a-Fe2O3 hollow nanohorns on the CNT backbone for superior lithium storage c
Magnetic-？eld induced formation of 1D Fe3O4/C/CdS coaxial nanochains as highly ef？cient and reusable
Facile one-pot synthesis of uniform TiO2-Ag hybrid hollow spheres with enhanced photocatalytic activ
Facile Low-Temperature Synthesis of Carbon Nanotube/TiO2 Nanohybrids with Enhanced Visible-Light-Dri
One-pot solvothermal synthesis of multi-shelled α-Fe2O3 hollow spheres with enhanced visible-light p
Facile growth of ZnO nanocrystals on nitrogen-doped carbon nanotubes for visible-light photodegradat
Facile one-pot synthesis of uniform TiO2–Ag hybrid hollow spheres with enhanced photocatalytic activ
Uniform hamburger-like mesoporous carbon-incorporated ZnO nanoarchitectures: One-pot solvothermal sy
Direct coating ZnO nanocrystals onto 1D Fe3O4/C composite microrods as highly efficient and reusable
Solvothermal Synthesis of Nickel Glycolate Polymer and NiO Microtubes and Their Cr(Ⅵ) Absorbing Prop
Controllable one-pot synthesis of various one-dimensional Bi2S3 nanostructures and their enhanced vi
Magnetic-field induced formation of 1D Fe3O4/C/CdS coaxial nanochains as highly efficient and reusab
A magnetically separable photocatalyst based on nest-likeg-Fe2O3/ZnO double-shelled hollow structure
Carbon nanocoating: an effective nanoreactor towards well-defined carbon-coated GaN hollow nanospind
Assembling carbon-coated alpha-Fe2O3 hollow nanohorns on the CNT backbone for superior lithium stora
Facile Formation of Mesoporous BiVO4/Ag/AgCl Heterostructured Microspheres with Enhanced Visible-Lig
Facile fabrication of mesoporous BiOCl/(BiO)2CO3/Bi2O3 ternary flower-like heterostructured microsph
Facile synthesis of Z-scheme Ag2CO3/Ag/AgBr ternary heterostructured nanorods with improved photosta
Facile formation of Ag2WO4/AgX (X = Cl, Br, I) hybrid nanorods withenhanced visible-light-driven pho
Formation of MS–Ag and MS (M=Pb, Cd, Zn) nanotubes viamicrowave-assisted cation exchange and their e
Facile preparation of 2D sandwich-like CdS nanoparticles/nitrogen-doped reduced graphene oxide hybri
Electrostatic self-assembly of TiO2 nanoparticles onto carbon spheres with enhanced adsorption capab
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