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东平湖水源地水环境健康风险初步评价
  • ISSN号:1009-6094
  • 期刊名称:安全与环境学报
  • 时间:2011
  • 页码:111-115
  • 分类:X824[环境科学与工程—环境工程]
  • 作者机构:[1]聊城大学环境与规划学院,山东聊城252000, [2]华东师范大学资源与环境科学学院,上海200062
  • 相关基金:国家自然科学基金项目(40772209,41072258,40901276);山东省自然科学基金项目(ZR2010DL007);聊城大学科研基金项目(X09043)
  • 相关项目:全新世以来东平湖变迁与黄河洪水关系及动力机制研究
中文摘要:

为了解东平湖水环境中污染物的分布特征、来源及健康风险,于2010年12月(冬季)环湖均匀采集了33个表层水样,分析了其N、P营养盐和Hg、As的质量浓度,并应用健康风险评价模型进行初步评价。结果表明,以《地表水环境质量标准》(GB 3838—2002)Ⅲ类水标准值为评价标准,总P和Hg质量浓度的超标率分别为30.3%和48.4%。湖东区、东南区总P质量浓度较高,可能是由于大汶河的输入和底泥的二次释放;沿湖四周Hg质量浓度高于湖心区,这可能与库区燃煤和垃圾焚烧有关。As通过饮水途径产生的致癌风险平均值为2.18×10-6 a-1,高于美国国家环保局(US EPA)推荐的1.0×10-6 a-1的最大可接受风险水平,超标率为77.4%;而非致癌物Hg、NH4+-N和NO3--N的健康风险等级为10-12~10-9 a-1。研究表明,东平湖水环境中致癌物As的健康风险值远大于非致癌物质,建议对As作进一步的溯源调查。

英文摘要:

The present paper is concerned about our investigation and analysis of the concentrations of the total 33 surface water samples collected uniformly around the water-coming sources of Dongping Lake in December, 2010. For our research purpose, we have done preliminary health risk assessment involved with the pollutants for drinking water by using the models of US EPA. The results of our preliminary assessment show that the concentrations of the total phosphorus and mercury exceed 30.3% and 48.4% of the contrast samples of type III standard values of the GB 3838—2002 National Environmental Quality Standards for Surface Water respectively, whereas pH value , the concentrations of DO, NH4+-N and As stay below the above-said standards. To be more exact, we have found the total phosphorus much higher than normal in the east and southeast areas of the lake, which implies that the sources of total phosphorus are likely to originate from Dawen River, the unique river merging into the lake from its southeastern side as well as the secondary release of phosphorus from the lake deposits. As to mercury, its concentrations were detected on the whole higher surrounding the lake than in its central area, which may account for the coal burning and garbage incineration in the villages around the lake. In addition, the individual carcinogenic risk value is likely to be caused by As through drinking water at the rate of 9.08×10-8-4.28×10-6 a-1 with an average of 2.18×10-6 a-1, higher than 1.0×10-6 a-1 of the up-limit tolerate level recommended by US EPA but lower than the standard 5.0×10-5 a-1 recommended by ICRP. It is particularly necessary to stress that the ratio of the samples with carcinogenic risk caused by As is also 77.4% above the standard 1.0×10-6 a-1, the maximum risk found in the sample collected near the inlet of Dawen River. Moreover, the non-carcinogens discovered stand in the order of Hg (3.07×10-10 a-1)〉NO3--N (1.39×10-10 a-1)〉NH4+-N (7.07×10-11 a-1) and the total risk was 1.38×10-10-

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期刊信息
  • 《安全与环境学报》
  • 北大核心期刊(2011版)
  • 主管单位:中国兵器工业集团公司
  • 主办单位:北京理工大学 中国环境科学学会 中国职业安全健康协会
  • 主编:冯长根
  • 地址:北京市海淀区中关村南大街5号
  • 邮编:100081
  • 邮箱:aqyhjxb@263.net;aqyhjxb@wuma.com.cn
  • 电话:010-68913997
  • 国际标准刊号:ISSN:1009-6094
  • 国内统一刊号:ISSN:11-4537/X
  • 邮发代号:2-770
  • 获奖情况:
  • 获首届《CAJ-CD》执行优秀期刊奖,中国科技论文统计源期刊
  • 国内外数据库收录:
  • 美国化学文摘(网络版),中国中国科技核心期刊,中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版)
  • 被引量:17182