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沉积氧压对La_0.8Sr_0.2MnO_3/0.7wt%Nb:SrTiO_3异质结的整流伏安特性及输运性的调控
  • ISSN号:1000-3258
  • 期刊名称:《低温物理学报》
  • 时间:0
  • 分类:TN713.1[电子电信—电路与系统]
  • 作者机构:[1]安徽省信息材料与器件重点实验室,安徽大学物理与材料科学学院,合肥230039
  • 相关基金:国家自然科学基金(批准号:11174001);安徽省教育厅重点科研基金(批准号:KJ2009A124)资助课题.
中文摘要:

采用脉冲激光沉积法在(100)0.7wt%Nb:SrTi03(NSTO)衬底上制备了La0.8Sr0.2Mn03(LSMO)/NSTO(100)异质结,仔细研究了原位沉积氧压和真空退火对LSMO/NSTO异质结的结构及其整流伏安特性的调控.X-射线线性扫描和原子力显微镜测量显示,低氧压制备的LSMO/NST0(100)异质结具有良好的外延结构和平整的表面.电流-电压(I-V)盐线显示,沉积氧压为100mTorr的异质p~n结展现出极好的整流伏安特性;而氧压为240mTorr的异质p~n结平缓增加的电流可解释为异质P~n结在界面处晶格缺陷的增加.作为对比,沉积氧压调控的LSMO/SrTiO3(100)薄膜的输运性也被研究.电阻率结果显示,低氧压制备的LSMO薄膜,其电阻率的增加及金属-半导体转变温度L的降低归因于氧空位增加诱导的Mn4+离子减少及MnO6八面体的畸变.

英文摘要:

Heteroepitaxial junction composed of the La0. 8Sr0. 2 MnO3 (LSMO) and the (100) 0. 7wt Nb: SrTiOa (NSTO) has been fabricated by pulsed-laser deposition. The effect of the in-situ deposition oxygen pressures and the annealed in vacuum on the structure and the rectifying current-voltage behaviors in LSMO/NSTO(100) heterojunctions were carefully studied. X-ray linear scans and atomic force microscope (AFM) patterns indicate that the LSMO/NSTO(100) heterojunctions grown at lower oxygen pressures have a better epitaxial quality and the smooth surface. The result of current-voltage (I-V) curves shows that the p-n junction grown at oxygen pressure of 100 mTorr exhibits an excellent rectifying behavior, but the p-n junction grown at a pressure of 240 mTorr displays a flat the I-V curves, which is ascribed to the increase of the lattice defects in pun junction interface. As a contrast,the transport properties of epitaxial LSMO/SrTiO3 (100) films were also studied by the modulating deposition oxygen pressures. The resistivity measurements shown that the increase of overall resistivity and the low of metal-insulator transition temperatures Tp in the LSMO films grown at lower oxygen pressures can be aseribed to the oxygen vaeancy inducing the decrease of Mn4+ ions as well as the distortion of MnO6 octahedron

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期刊信息
  • 《低温物理学报》
  • 北大核心期刊(2011版)
  • 主管单位:中国科学院
  • 主办单位:中国科学技术大学
  • 主编:赵忠贤
  • 地址:安徽省合肥市金寨路96号
  • 邮编:230026
  • 邮箱:LiBiyou@ustc.edu.cn
  • 电话:0551-3601359
  • 国际标准刊号:ISSN:1000-3258
  • 国内统一刊号:ISSN:34-1053/O4
  • 邮发代号:26-136
  • 获奖情况:
  • 国内外数据库收录:
  • 美国化学文摘(网络版),日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国北大核心期刊(2000版)
  • 被引量:1577