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南四湖内源氮磷释放的对比研究
  • ISSN号:0253-2468
  • 期刊名称:环境科学学报
  • 时间:2013.2
  • 页码:487-493
  • 分类:X524[环境科学与工程—环境工程]
  • 作者机构:[1]山东省水土保持与环境保育重点实验室,临沂大学资源环境学院,临沂276005, [2]山东师范大学人口·资源与环境学院,济南250014
  • 相关基金:山东省中青年科学家科研奖励基金(No.2009BSA13006); 临沂大学博士科研启动基金(No.BS201006); 国家自然科学基金(No.21207058),致谢:中国科学院南京地理与湖泊与研究所为本研究提供沉积物柱状采样器及Peeper间隙水采集器,山东师范大学爨景波同学和王千锁同学、临沂大学的张旭同学在样品采集和沉积物切样时,给予帮助,在此一并表示感谢.
  • 相关项目:风浪扰动下南四湖沉积物Hg和Pb的动态迁移及其定量化研究
中文摘要:

采用柱状沉积物采样器和Peeper间隙水采集器分别于2011年8月获取南四湖不同湖区原位柱状沉积物和间隙水,通过原柱样静态释放实验及间隙水分子扩散模型对其氮磷释放规律进行了研究.结果表明,南四湖不同湖区夏季氮磷界面交换速率差异显著,静态释放实验沉积物NH4^+-N和PO4^3--P的释放速率分别为3.1~10.3mg·m^-2·d^-1和0.3~2.7mg·m^-2·d^-1,总体呈北高南低的趋势,南阳湖明显大于其他各湖区,这与其距离济宁市区较近,沉积物受污染较重有关.Peeper法与离心法分别获取不同湖区间隙水,利用分子扩散模型计算出NH4^+-N和PO4^3--P的释放速率分别为3.69~4.51mg·m^-2·d^-1、0.24~0.66mg·m^-2·d^-1和2.54~4.16mg·m^-2·d^-1、0.04~0.51mg·m^-2·d^-1,同一采样点,Peeper法计算出释放速率比传统离心法高出约20%.通过静态释放实验获得的NH4^+-N和PO4^3--P释放速率(R)在空间分布上与间隙水分子扩散模型计算出的结果相一致,但前者明显大于后者,将其进行比较,氮和磷的R/F值分别为0.84~2.64和2.03~13.79,表明原柱样静态模拟实验进行内源释放速率估算时,可能比分子扩散模型法计算的结果更接近于实际情况.

英文摘要:

)Intact sediments and interstitial water were collected by sediment sampler and Peeper (pore water equilibriums) from different zones of Nansi Lake in August 2011, and the release of nitrogen and phosphorus in sediments were studied through static incubation and interstitial water molecule diffusion model. Results showed that nitrogen and phosphorus releasing rates from sediments were significantly different between zones of Nansi Lake in summer, with a general north-to-south decreasing trend. The release rates of NH4^+-N and PO4^3--P through static incubation were 3.1-10.3 mg · m^-2 · d^-1 and 0.3-2.7 mg · m^-2 · d^-1, respectively. The release rates of NH4^+-N and PO4^3--P from Nanyang Lake were significantly greater than other Lakes and this may be due to the serious pollution from the nearby Jining City to the Northern Nansi Lake. Centrifugation and Peeper method were used to obtain porewater in different sampling areas of Nansi Lake, and the releasing rates of sediment NH4^+-N and PO4^3--P estimated by Fick′s Law were 3.69-4.51 mg · m^-2 · d^-1, 0.24-0.66 mg · m^-2 · d^-1 and 2.54-4.16 mg · m-2 · d^-1, 0.04-0.51 mg · m^-2 · d^-1, respectively. The releasing rates calculated by Peeper were about 20% higher than those by conventional centrifugal method. The spatial distributions of NH4^+-N and PO4^3--P releasing rates estimated by static incubations and interstitial water molecule diffusion model were consistent, with the releasing rates of NH4^+-N much higher than PO4^3--P. The R/F value of NH4^+-N and PO4^3--P were 0.84-2.64 and 2.03-13.79, respectively. The results indicated that the release rates obtained by static incubations with intact sediment cores may be closer to the actual situation than those by interstitial water molecule diffusion model.

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期刊信息
  • 《环境科学学报》
  • 中国科技核心期刊
  • 主管单位:中国科学院
  • 主办单位:中国科学院生态环境研究中心
  • 主编:汤鸿霄
  • 地址:北京2871信箱
  • 邮编:100085
  • 邮箱:hjkxxb@rcees.ac.cn
  • 电话:010-62941073
  • 国际标准刊号:ISSN:0253-2468
  • 国内统一刊号:ISSN:11-1843/X
  • 邮发代号:82-625
  • 获奖情况:
  • 国内外数据库收录:
  • 美国化学文摘(网络版),荷兰地学数据库,荷兰文摘与引文数据库,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),英国英国皇家化学学会文摘,中国北大核心期刊(2000版)
  • 被引量:56074