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黄山地区春夏季气溶胶离子组分及其对云微物理特征的影响
  • ISSN号:0577-6619
  • 期刊名称:气象学报
  • 时间:0
  • 页码:-
  • 分类:P401[天文地球—大气物理学与大气环境;天文地球—大气科学及气象学]
  • 作者机构:[1]南京信息工程大学气象灾害教育部重点实验室,南京210044, [2]南京信息工程大学中国气象局大气物理与大气环境重点开放实验室,南京210044
  • 相关基金:资助课题:国家自然科学基金项目(41030962)、江苏高校优势学科建设工程资助项目(PAPD).
  • 相关项目:我国南方地形云和气溶胶相互作用的观测和理论研究
中文摘要:

利用2009年5—8月在华东地区高山——黄山顶取得的气溶胶和云微物理参数观测资料以及同期气溶胶离子成分数据,结合多种化学组分气溶胶绝热气块分档云模式,研究了黄山地区多化学组分气溶胶对云凝结核和云微物理特征的影响。气团轨迹和气溶胶离子成分的分析结果表明,3种气团影响着黄山地区气溶胶的化学组分,即北方大陆气团气溶胶富含CaCO3,局地污染气团气溶胶以可水溶性无机盐((NH4)2SO4、NH4NO3)为主,而变性混合海洋性气团气溶胶中NaCI较多。数值模拟结果显示,在气溶胶谱一定时,不同天气形势下黄山气溶胶的化学组分的差异会对云微物理特征产生不同的影响。同一上升速度下实际多组分气溶胶模拟的云滴数浓度大于纯硫酸铵,主要体现在云滴谱第1个峰值3.3μm之前;气块上升速度低于0.7m/s时,含有较多不可水溶物质的混合气溶胶对云滴数浓度的影响较大;上升速度大于0.7m/s时,气块中可凝结水增多,海盐对云滴数浓度增加的效果更显著。多组分气溶胶模拟云滴谱较纯硫酸铵窄,其中,北方气团方案造成云滴谱变窄的程度高于混合气团方案;而模拟的云滴数目增多,造成云滴有效半径减小,云光学厚度和反照率增加,将会对暖云降水及辐射效应产生不同的影响。

英文摘要:

The aerosol components and cloud microphysical parameters were measured at a high-altitude background station on the summit of the Mr. Huang from May to August 2009, and were used as input to a multi-chemical-component (MCC) bin-resolved cloud parcel model to investigate the influence of MCC aerosols on the cloud condensation nuclei (CCN) and cloud microphysics. The results from the back trajectory cluster and aerosol ionic composition analysis show that there were three types of air masses that affected the chemical composition of the aerosol particles, including the northern continental, local polluted, and mixed transformation maritime air mass, with characteristic substance of CaCO3, soluble salts ((NH4)2 SO4, NH4 NOa), as well as NaC1, respectively. The numerical simulation results show that the effects of aerosol chemical compositions on cloud microphysical processes varied with weather conditions for the same aerosol distribution. MCC aerosols led to higher cloud droplet number concentration (CDNC) than pure ammonium sulfate aerosols under the same updraft velocity, mainly reflected in more droplets with sizes less than 3.3 μm. It is also shown that inclusion of the insoluble component CaCO3 has more significant influence on the CDNC when the updraft velocity is lower than 0. 7 m/s; other- wise, NaC1 dominated the droplet activation process with the increasing condensable water. The MCC aerosols resulted in relatively narrow cloud droplet spectrum than pure ammonium sulfate aerosols, especially when the area is influenced by the northern continental air mass. In the latter case, MCC aerosols led to enhanced the cloud droplet number, cloud optical thickness and cloud albedo, and decreased the droplet effective radius, and therefore, may have different effects to warm precipitation and atmospheric radiation compared with other types of air masses.

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期刊信息
  • 《气象学报》
  • 北大核心期刊(2011版)
  • 主管单位:中国气象局
  • 主办单位:中国气象学会
  • 主编:丁一汇
  • 地址:北京市中关村南大街46号
  • 邮编:100081
  • 邮箱:qxxb@cms1924.org
  • 电话:010-68406942
  • 国际标准刊号:ISSN:0577-6619
  • 国内统一刊号:ISSN:11-2006/P
  • 邮发代号:2-368
  • 获奖情况:
  • 第三届中国出版政府奖提名奖
  • 国内外数据库收录:
  • 美国化学文摘(网络版),日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国北大核心期刊(2000版)
  • 被引量:21756