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扰动强度对太湖沉积物中磷释放及其形态转化的影响
  • ISSN号:0250-3301
  • 期刊名称:环境科学
  • 时间:0
  • 页码:2614-2620
  • 分类:X131.2[环境科学与工程—环境科学]
  • 作者机构:[1]苏州科技学院环境科学与工程学院,苏州215011
  • 相关基金:国家自然科学基金项目(50908154,50938005)
  • 相关项目:城市水体底泥资源化用于水体磷的吸收和内源磷固定的机制研究
中文摘要:

通过室内试验模拟了太湖沉积物在不同扰动强度下的悬浮过程,研究了沉积物扰动强度对磷释放及其形态转化的影响.结果表明,较高扰动强度下(相当于太湖风速12 m.s-1),水体中不同形态磷(总磷、颗粒态磷、溶解性总磷)含量均高于较低扰动强度(相当于太湖风速8 m.s-1).其中,两者分别扰动1h后,总磷和颗粒态磷分别达到0.950 mg.L-1、0.384 mg.L-1和0.882 mg.L-1、0.328 mg.L-1,该水平保持到试验结束.然而,溶解性总磷则呈逐渐降低的趋势.这主要归因于悬浮物的吸附和微生物的快速利用.较高和较低扰动强度下,悬浮物上总磷(Tot-P)分别增加了10 mg.kg-1(平均值)和60 mg.kg-1(平均值).较高扰动强度下铁铝结合态磷的变化恰好说明了形态磷间存在转化趋势.因为铁铝结合态磷增加了85.7 mg.kg-1(平均值),明显高于Tot-P的实测值(10 mg.kg-1,平均值)和理论值(27 mg.kg-1,平均值),说明有其它形态磷转化成铁铝结合态磷.弱吸附态磷和钙结合态磷含量的降低正说明这一点.这显示在扰动状态下,不同形态磷之间至少发生了以水为媒介的间接性转化.

英文摘要:

Lab-scale experiments were conducted to investigate the effect of sediment disturbance under different intensity conditions on phosphorus(P) release and sedimentary P transformation.The sediments came from Taihu Lake.The results show that the concentrations of total P(TP),particulate P(PP) and dissolved total P(DTP) in the overlying water under high intensity conditions(equal to the force of 12 m·s-1 wave velocity on the bottom sediment in Taihu Lake) were higher than those under low intensity conditions(equal to the force of 8 m·s-1).The concentrations of TP and PP were up to 0.950 mg·L-1,0.384 mg·L-1and 0.882 mg·L-1,0.328 mg·L-1 for both intensities after 1 h and then the levels kept unchanged almost till the end of the experiments.However,the DTP decreased gradually.It is attributed to the adsorption by suspended sediments and quick uptake by microorganisms.Under both intensities conditions,the Tot-P of the suspended particulate matter(SPM) due to disturbance increased by 10 mg·kg-1(mean during 0-12 h) and 60 mg·kg-1(mean during 0-12 h).The changes of Fe/Al-P during the experiment(0-12 h) verified the transformation trend between sedimentary P forms in the SPM under high intensity.Because the net increase(85.7 mg·kg-1,mean during 0-12 h) was higher than the measured value(10 mg·kg-1,mean during 0-12 h) and the theoretically calculated value(27 mg·kg-1,mean during 0-12 h).It suggests that other sedimentary P forms were transformed into Fe/Al-P.Correspondingly,the decrease of NH4Cl-P and HCl-P can verify this.It suggested that sediment disturbance might induce the indirect transformation between sedimentary P forms by the assistance of overlying water.

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期刊信息
  • 《环境科学》
  • 中国科技核心期刊
  • 主管单位:中国科学院
  • 主办单位:中国科学院生态环境研究中心
  • 主编:赵进才
  • 地址:北京市2871信箱(海淀区双清路18号)
  • 邮编:100085
  • 邮箱:hjkx@rcees.ac.cn
  • 电话:010-62941102 62849343
  • 国际标准刊号:ISSN:0250-3301
  • 国内统一刊号:ISSN:11-1895/X
  • 邮发代号:2-821
  • 获奖情况:
  • 在全国第一届和第二届优秀科技期刊评比中分别荣获...,二次荣获中国科学院优秀期刊评比一等奖,荣获中国期刊方阵双奖期刊荣誉
  • 国内外数据库收录:
  • 俄罗斯文摘杂志,美国化学文摘(网络版),荷兰文摘与引文数据库,美国工程索引,美国生物医学检索系统,美国剑桥科学文摘,美国生物科学数据库,英国动物学记录,日本日本科学技术振兴机构数据库,中国中国科技核心期刊,中国北大核心期刊(2004版),中国北大核心期刊(2008版),中国北大核心期刊(2011版),中国北大核心期刊(2014版),中国北大核心期刊(2000版)
  • 被引量:69962